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Glasses are nonequilibrium solids with properties highly dependent on their method of preparation. In vapor-deposited molecular glasses, structural organization could be readily tuned with deposition rate and substrate temperature. Here, we show that the atomic arrangement of strong network-forming GeO 2 glass is modified at medium range (<2 nm) through vapor deposition at elevated temperatures. Raman spectral signatures distinctively show that the population of six-membered GeO 4 rings increases at elevated substrate temperatures. Deposition near the glass transition temperature is more efficient than postgrowth annealing in modifying atomic structure at medium range. The enhanced medium-range organization correlates with reduction of the room temperature internal friction. Identifying the microscopic origin of room temperature internal friction in amorphous oxides is paramount to design the next-generation interference coatings for mirrors of the end test masses of gravitational wave interferometers, in which the room temperature internal friction is a main source of noise limiting their sensitivity.more » « less
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Vajente, Gabriele ; Yang, Le ; Davenport, Aaron ; Fazio, Mariana ; Ananyeva, Alena ; Zhang, Liyuan ; Billingsley, Garilynn ; Prasai, Kiran ; Markosyan, Ashot ; Bassiri, Riccardo ; et al ( , Physical Review Letters)null (Ed.)
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Lalande, Émile ; Lussier, Alexandre W. ; Lévesque, Carl ; Ward, Marianne ; Baloukas, Bill ; Martinu, Ludvik ; Vajente, Gabriele ; Billingsley, Garilynn ; Ananyeva, Alena ; Bassiri, Riccardo ; et al ( , Journal of Vacuum Science & Technology A)